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Study of corrosion behavior of virgin and recycled Pb anodes used in zinc electrowinning industry

Shima Nakisa (Faculty of Material Engineering, Sahand University of Technology, Tabriz, Iran)
Naghi Parvini Ahmadi (Faculty of Material Engineering, Sahand University of Technology, Tabriz, Iran)
Javad Moghaddam (Faculty of Material Engineering, Sahand University of Technology, Tabriz, Iran)
Habib Ashassi-Sorkhabi (University of Tabriz, Tabriz, Iran)

Anti-Corrosion Methods and Materials

ISSN: 0003-5599

Article publication date: 14 October 2020

Issue publication date: 4 December 2020

200

Abstract

Purpose

The composition and corrosion behaviors of recycled and virgin Pb anode were investigated in industrial zinc electrowinning solution with different methods. The purpose of this study is the illustration of good anticorrosion activity of virgin Pb anodes compared to recycled one in industrial operation, while the compositions of both of them are the same which obtained from quantmetry method.

Design/methodology/approach

Its corrosion properties and electrocatalytic activity toward oxygen evolution reaction were appraised using potentiodynamic polarization, electrochemical impedance spectroscopy, galvanostatic polarization and ionic equilibrium methods. In addition, composition of anodes investigated with X-ray photoelectron spectroscopy (XPS) method. The surface composition of samples was studied via X-ray diffractogram (XRD).

Findings

The results indicate that the anodes display different anodic behaviors during the galvanostatic polarization. Virgin Pb anode shows a “potential reduction” about 320 mV lower than recycled Pb anode after 6 h of polarization; also, the stable potential after 72 h for virgin Pb anode is 100 mV lower than recycled Pb anode. Also, The XPS results show a trace amount of Cl in recycled anodes which cause the more corrosion activity. XRD results indicate that virgin Pb anodes have been covered by more oxides than recycled anodes after 72 h of electrowinning.

Originality/value

The treatment of corrosion behavior by virginity has not been detected by any researchers yet. Therefore, it is imperative to study the corrosion behavior and exact composition analysis of virgin and recycled Pb anodes to comprehension of them. This paper fulfills this need.

Keywords

Acknowledgements

The authors gratefully acknowledge the Zanjan Zinc Khales Sazan Industries Company (ZZKI Co.) for the financial and technical support of this work.

Citation

Nakisa, S., Parvini Ahmadi, N., Moghaddam, J. and Ashassi-Sorkhabi, H. (2020), "Study of corrosion behavior of virgin and recycled Pb anodes used in zinc electrowinning industry", Anti-Corrosion Methods and Materials, Vol. 67 No. 6, pp. 529-536. https://doi.org/10.1108/ACMM-04-2017-1787

Publisher

:

Emerald Publishing Limited

Copyright © 2020, Emerald Publishing Limited

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