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The purpose of this study is to perform a detailed review on the numerical modeling of multiphase and multicomponent flows in microfluidic system using phase-field method. The phase-field method is of emerging importance in numerical computation of transport phenomena involving multiple phases and/or components. This method is not only used to model interfacial phenomena typical to multiphase flows encountered in engineering and nature but also turns out to be a promising tool in modeling the dynamics of complex fluid-fluid interfaces encountered in physiological systems such as dynamics of vesicles and red blood cells). Intrinsically, a priori unknown topological evolution of interfaces offers to be the most concerning challenge toward accurate modeling of moving boundary problems. However, the numerical difficulties can be tackled simultaneously with numerical convenience and thermodynamic rigor in the paradigm of the phase field method.

The phase-field method replaces the macroscopically sharp interfaces separating the fluids by a diffuse transition layer where the interfacial forces are smoothly distributed. As against the moving mesh methods (Lagrangian) for the explicit tracking of interfaces, the phase-field method implicitly captures the same through the evolution of a phase-field function (Eulerian). In contrast to the deployment of an artificially smoothing function for the interface as used in the volume of a fluid or level set method, however, the phase-field method uses mixing free energy for describing the interface. This needs the consideration of an additional equation for an order parameter. The dynamic evolution of the system (equation for order parameter) can be described by Allen–Cahn or Cahn–Hilliard formulation, which couples with the Navier–Stokes equation with the aid of a forcing function that depends on the chemical potential and the gradient of the order parameter.

In this review, first, the authors discuss the broad motivation and the fundamental theoretical foundation associated with phase-field modeling from the perspective of computational microfluidics. They subsequently pinpoint the outstanding numerical challenges, including estimations of the model-free parameters. They outline some numerical examples, including electrohydrodynamic flows, to demonstrate the efficacy of the method. Finally, they pinpoint various emerging issues and futuristic perspectives connecting the phase-field method and computational microfluidics.

This paper gives unique perspectives to future directions of research on this topic.